“…Giant dielectric permittivity materials such as CaCu 3 Ti 4 O 12 (CCTO) and isostructural ACu 3 Ti 4 O 12 -oxides [ [1] , [2] , [3] , [4] , [5] , [6] , [7] , [8] , [9] , [10] ], CuO [ 11 ], co-doped NiO-based oxides [ 12 , 13 ], AFe 1/2 B 1/2 O 3 (A = Ca, Sr, Ba; B = Sb, Ta, Nb) [ 14 ], co-doped TiO 2 -based oxides [ [15] , [16] , [17] , [18] , [19] , [20] , [21] , [22] ], co-doped SrTiO 3 -based oxides [ 23 ], and Ln 2-x Sr x NiO 4 ( Ln = La, Nd, and Sm) ( Ln SNO) ceramics [ [24] , [25] , [26] , [27] , [28] , [29] , [30] ], have been widely investigated in recent years. These giant dielectric materials (or colossal-permittivity materials) can exhibit extreme values of dielectric permittivity (ε′) of approximately 10 4 –10 6 compared to those of ferroelectric materials ( e.g.…”