2023
DOI: 10.1021/acsphotonics.3c01315
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Abundant Evolution Processes of Polaron-Pairs and Exciplex States with Various Electron–Hole Coupling Distances in Exciplex-Based OLEDs by Modifying Device Hole-Injection Abilities

Xi Zhao,
Jing Chen,
Lihong Cheng
et al.

Abstract: Intersystem crossing (ISC) and reverse ISC (RISC) between singlet and triplet polaron-pairs (PP) and exciplex (EX) states, triplet-charge annihilation (TCA), and triplet−triplet annihilation (TTA) are well-known key spin-mixing processes in EX-based organic light-emitting diodes (EX-OLEDs) for improving the device optoelectronic performances. These microscopic processes usually show normal current dependencies; i.e., ISC and RISC weaken while TCA and TTA enhance with increasing bias current, respectively. Here… Show more

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