We identify a novel regime of soliton-plasma interactions in which high-intensity ultrashort pulses of intermediate soliton order undergo coherent plasma-induced fission. Experimental results obtained in gasfilled hollow-core photonic crystal fibers are supported by rigorous numerical simulations. The cumulative blueshift of higher-order input solitons with ionizing intensities results in pulse splitting before the ultimate self-compression point, leading to the generation of robust pulse pairs with PHz bandwidths. The novel dynamics closes the gap between plasma-induced adiabatic soliton compression and modulational instability.PACS numbers: 42.81. Dp, 42.65.Re, 32.80.Fb The interaction of ultrashort laser pulses with photoinduced plasmas has been the subject of intense research, and its understanding is of fundamental importance in many different fields, for example optical filamentation [1] and attosecond physics [2]. The field has been mostly studied in free space [3] and fiber capillaries [4]. In both these cases, however, spurious spatial effects complicate the dynamics and control over the propagation of the laser pulses is limited. Over the past few years, gas-filled hollow-core photonic crystal fiber [5] (PCF) has matured as an ideal platform for studying the interaction of laser light with matter. The tight confinement of high-intensity femtosecond pulses in a single spatial mode with precisely controllable anomalous dispersion allows established soliton dynamics to be extended into the strong-field regime [6], opening up unique possibilities. For the first time, it has been possible to study how optical solitons interact with plasmas over long pathlengths and broad frequency ranges in a well-controlled environment, as well as effects such as plasma-induced blue-shifting [7,8], adiabatic soliton compression [9] and modulational instability (MI) [10].In previous work, soliton-plasma interactions were mainly studied in the regimes of low and very high soliton order. Here we investigate high-intensity ultrashort solitons of intermediate order, and demonstrate novel coherent plasma-induced fission, leading to pulse splitting and the production of robust pulse pairs of PHz bandwidth that co-propagate phase-locked over cm-long distances. We furthermore show that the regimes of soliton-based pulse compression [11][12][13], supercontinuum generation [14,15], dispersive wave (DW) emission [16,17], soliton blue-shifting and plasma-induced fission can be accessed in a single system, simply by changing the input pulse energy. The findings are of great practical interest as hollow-core PCF-based pulse manipulation schemes evolve into a highly-demanded asset in modern high-repetition rate laser systems [18,19].In the experiment, an 8-cm-long kagomé-type PCF with 36 μm core diameter and 200 nm core wall thickness was placed in a gas-cell filled with 2 bar of Kr. It was pumped by 28-fs-long (full-width-half-maximum -FWHM) pulses at ~0.29 PHz (1.03 μm) with up to 13.2 μJ pulse energy at a repetition rate of 151 kHz....