“…Constructing gradient nanostructures (GNSs) have been proven to be a good strategy for enhancing the mechanical properties of metals and alloys inspired by nature [1,2]. Over the past two decades, this strategy has been successfully applied in almost all types of structural metallic materials [3][4][5][6][7], such as Cu and Cu alloys [8,9], Mg alloys [10,11], and Ti alloys [12,13]. Several methods have been developed to prepare the gradient nanostructure, such as surface mechanical grinding treatment (SMGT) [3], surface mechanical attrition treatment (SMAT) [14], surface mechanical rolling treatment (SMRT) [15], laser shock peening (LSP) [16], ultrasonic surface rolling (USR), or ultrasonic nanocrystalline surface modification (UNSM) [17][18][19][20].…”