To obtain better trajectory tracking, a new synchronous control with sliding mode surface is proposed. Based on Kane equation, the dynamics model of a planar 2-DOF redundantly actuated parallel mechanism was formulated. With trajectory contour error, the synchronization error was defined and the sliding surface was determined. After dynamic equation linearization, a robust adaptive sliding mode synchronous controller was designed with stability analysis. After Matlab simulation, figures of tracking errors and synchronization errors changing with time compared with computed torque method were plotted. Results show that the robust adaptive sliding mode synchronous control can be able to achieve good trajectory tracking compared with computed torque controller.