Adjustable composition of self-supported amorphous Ni–Fe–P nanosheet decorated NiP microspheres for efficient and stable overall alkaline freshwater/seawater splitting

Lu, Shi-Yu; Wang, Ling; Wu, Chunjie; Zhang, Jun; Dou, Wenzhao; Hu, Tingting; Wang, Rong; Liu, Yin; Yang, Qian; Jin, Meng

doi:10.1039/d4qi00582a

Inorg. Chem. Front.

2024

DOI: 10.1039/d4qi00582a

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Adjustable composition of self-supported amorphous Ni–Fe–P nanosheet decorated NiP microspheres for efficient and stable overall alkaline freshwater/seawater splitting

Shi-Yu Lu,

Ling Wang,

Chunjie Wu

et al.

Abstract: Self-supported amorphous Ni–Fe–P nanosheet decorated NiP microspheres for efficient and stable overall alkaline freshwater/seawater splitting.

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Multihybridization for Enhancing Fe‐Ni Bimetal Electrocatalyst in Water Oxidation

Zhang,

Zhou,

Wang

et al. 2024

Advanced Energy Materials

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Water electrolysis holds the promise of transforming electric‐power into hydrogen energy through a carbon free process and its widespread application highly depends on anodic oxygen evolution reaction (OER) efficiency. Transition metal‐based OER catalysts meet the requirements of long‐term development for cost effectiveness, and their performance can be improved by a variety of band electronic structure modulating methods. Herein, a multihybridization strategy is proposed, i.e., p‐d, s‐sp, and d‐d hybridization are emphasized together, which guides the design of an effective vanadium (V), boron (B)‐FeNiP catalyst. Density functional theory analysis reveals the existence of multihybridization and the difference between Fe and Ni in terms of hybridization strength, band configuration, and interfacial charge transfer. Specially, Fe and Ni sites are simultaneously optimized to their highest performance upon the dual B, V incorporation. As a result, the VB‐FeNiP catalyst displays outstanding OER performance, regarding a Tafel slope of 57.64 mV dec−1, an overpotential of 175 mV at 100 mA cm−2, and exceptional stability. Here the synergistic effect of multihybridization in the design of transition metal‐based catalysts is highlighted and the work in pursuit of effective way based on regulating band configuration to developing high performance OER catalysts would be evoked.

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Multihybridization for Enhancing Fe‐Ni Bimetal Electrocatalyst in Water Oxidation

Zhang,

Zhou,

Wang

et al. 2024

Advanced Energy Materials

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High/Low-Index Faceted PdNi Alloy Nanocrystals as Highly Active and Stable Electrocatalyst for Oxygen Reduction

Zhang,

Xu,

Luo

et al. 2025

Chemical Engineering Journal

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Ternary Ni:Fe- activated inert Cu-based electrocatalyst as efficient bifunctional electrocatalysts for water splitting

Lu,

Wu,

et al. 2025

Chemical Engineering Journal

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Adjustable composition of self-supported amorphous Ni–Fe–P nanosheet decorated NiP microspheres for efficient and stable overall alkaline freshwater/seawater splitting

Abstract: Self-supported amorphous Ni–Fe–P nanosheet decorated NiP microspheres for efficient and stable overall alkaline freshwater/seawater splitting.

Cited by 5 publications

References 51 publications

Multihybridization for Enhancing Fe‐Ni Bimetal Electrocatalyst in Water Oxidation

Multihybridization for Enhancing Fe‐Ni Bimetal Electrocatalyst in Water Oxidation

High/Low-Index Faceted PdNi Alloy Nanocrystals as Highly Active and Stable Electrocatalyst for Oxygen Reduction

Ternary Ni:Fe- activated inert Cu-based electrocatalyst as efficient bifunctional electrocatalysts for water splitting

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