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NRC Publications Archive Archives des publications du CNRCThis publication could be one of several versions: author's original, accepted manuscript or the publisher's version. / La version de cette publication peut être l'une des suivantes : la version prépublication de l'auteur, la version acceptée du manuscrit ou la version de l'éditeur. For the publisher's version, please access the DOI link below./ Pour consulter la version de l'éditeur, utilisez le lien DOI ci-dessous.http://dx.doi.org/10.1016/j.cemconres. 2004.05.012 Cement and Concrete Research, 34, 9, pp. 1717Research, 34, 9, pp. -1724Research, 34, 9, pp. , 2004 LDH, and CaAl2NS LDH produced a tilted orientation of NBA and 26NS anions in the interlayer space, while 2NS anions induced a perpendicular bilayer arrangement.Materials characterization was carried out using X-ray diffraction, IR-spectroscopy, thermal analysis and Scanning Electron Microscopy. These preliminary results open up a new direction towards the synthesis of nanocomposites using polymeric entities and layered materials for future applications in cement and concrete science, e.g. control of the effect of admixtures on the kinetics of cement hydration by programming their temporal release.