Advancements and prospects of perovskite-based fuel electrodes in solid oxide cells for CO<sub>2</sub> electrolysis to CO

Xu, Ruijia; Liu, Shuai; Yang, Meiting; Yang, Guangming; Luo, Zhixin; Ran, Ran; Zhou, Wei; Shao, Zongping

doi:10.1039/d4sc03306j

Chem. Sci.

2024

DOI: 10.1039/d4sc03306j

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Advancements and prospects of perovskite-based fuel electrodes in solid oxide cells for CO₂ electrolysis to CO

Ruijia Xu,

Shuai Liu,

Meiting Yang

et al.

Abstract: Developments and prospects for solid oxide cells using a perovskite-based fuel electrode for CO2 electrolysis to CO.

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Cited by 6 publications

References 177 publications

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Recent Advances and Challenges in Perovskite‐Based Protonic Ceramic Electrolytes: Design Strategies and Fabrication Innovations

Nie,

Liu,

Xiao

et al. 2024

Adv Funct Materials

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Protonic ceramic electrochemical cells (PCECs) have received extensive research attention as full solid‐state, electrochemical devices that can interconvert electrical and chemical energies via rapid proton conduction at reduced temperatures. Nonetheless, the practical application of PCECs still faces numerous challenges. In addition to the development of electrode materials, the protonic ceramic electrolytes (PCEs), which are crucial for the performance and stability of PCECs, encounter issues such as poor sinterability, low ionic conductivity, and inadequate thermochemical matching. To address these obstacles, the design and optimization of protonic ceramic electrolytes have recently become essential research focuses in the field of PCECs. To achieve effective customization of the elemental composition, crystal structure, defect structure, ionic conductivity, and chemical stability, many candidates for electrolyte materials with various compositions have been proposed. This review also covers state‐of‐the‐art developments in PCE fabrication technologies, including powder synthesis, thin‐film deposition, more controllable sintering processes and interface treatments for structural integrity and ionic conductivity. This review comprehensively summarizes the most recent design approaches and optimization strategies for perovskite‐based protonic ceramic electrolyte materials and is crucial for advancing the commercialization of PCECs.

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Recent Advances and Challenges in Perovskite‐Based Protonic Ceramic Electrolytes: Design Strategies and Fabrication Innovations

Nie,

Liu,

Xiao

et al. 2024

Adv Funct Materials

View full text Add to dashboard Cite

show abstract

Proton diffusivity in protonic ceramic membrane for electrochemical methanation in molten salts

Tokushige,

Itoh,

Hachiya

2024

J Solid State Electrochem

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Electrosynthesizing high-value fuels from CO2 in solid oxide electrolysis cells: Fundamentals, advances, and perspectives

Yang,

Liu,

Liu

et al. 2024

Chinese Chemical Letters

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Advancements and prospects of perovskite-based fuel electrodes in solid oxide cells for CO₂ electrolysis to CO

Abstract: Developments and prospects for solid oxide cells using a perovskite-based fuel electrode for CO2 electrolysis to CO.

Cited by 6 publications

References 177 publications

Recent Advances and Challenges in Perovskite‐Based Protonic Ceramic Electrolytes: Design Strategies and Fabrication Innovations

Recent Advances and Challenges in Perovskite‐Based Protonic Ceramic Electrolytes: Design Strategies and Fabrication Innovations

Proton diffusivity in protonic ceramic membrane for electrochemical methanation in molten salts

Electrosynthesizing high-value fuels from CO2 in solid oxide electrolysis cells: Fundamentals, advances, and perspectives

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Advancements and prospects of perovskite-based fuel electrodes in solid oxide cells for CO2 electrolysis to CO

Abstract: Developments and prospects for solid oxide cells using a perovskite-based fuel electrode for CO2 electrolysis to CO.

Cited by 6 publications

References 177 publications

Recent Advances and Challenges in Perovskite‐Based Protonic Ceramic Electrolytes: Design Strategies and Fabrication Innovations

Recent Advances and Challenges in Perovskite‐Based Protonic Ceramic Electrolytes: Design Strategies and Fabrication Innovations

Proton diffusivity in protonic ceramic membrane for electrochemical methanation in molten salts

Electrosynthesizing high-value fuels from CO2 in solid oxide electrolysis cells: Fundamentals, advances, and perspectives

Contact Info

Product

Resources

About

Advancements and prospects of perovskite-based fuel electrodes in solid oxide cells for CO₂ electrolysis to CO