2023
DOI: 10.1002/tcr.202300044
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Advances in Ordered Architecture Design of Composite Solid Electrolytes for Solid‐State Lithium Batteries

Abstract: Solid electrolyte lithium batteries are the next generation of advanced energy devices. The incorporation of solid electrolytes can significantly improve the safety issue of lithium‐ion batteries. Organic‐inorganic composite solid electrolytes (CSE) are promising candidates for solid‐state batteries, but their application is mainly limited by low ionic conductivity. Many studies have shown that the architecture of ordered inorganic fillers in CSE can act as fast lithium‐ion transfer channels by auxiliary means… Show more

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Cited by 9 publications
(2 citation statements)
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References 104 publications
(224 reference statements)
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“…1–4 Conventional lithium-ion batteries, employing liquid organic electrolytes, inherently pose safety concerns due to their flammability, volatility, and susceptibility to leakage. 5–8 In response to these safety challenges, solid-state lithium batteries have emerged as a promising alternative, completely abandoning traditional organic electrolytes in favor of solid counterparts. This transformative shift not only addresses safety concerns, but also enhances performance characteristics.…”
Section: Introductionmentioning
confidence: 99%
“…1–4 Conventional lithium-ion batteries, employing liquid organic electrolytes, inherently pose safety concerns due to their flammability, volatility, and susceptibility to leakage. 5–8 In response to these safety challenges, solid-state lithium batteries have emerged as a promising alternative, completely abandoning traditional organic electrolytes in favor of solid counterparts. This transformative shift not only addresses safety concerns, but also enhances performance characteristics.…”
Section: Introductionmentioning
confidence: 99%
“…The pursuit of high-energy-density batteries is inevitable, driven by the growing demand for efficient energy storage solutions. Lithium metal stands out as a promising candidate for anode materials, boasting a high theoretical capacity of 3860 mA h/g and a low electrochemical potential of −3.04 V vs the standard hydrogen electrode. , Indeed, these characteristics position lithium metal as an ideal candidate for the next generation of rechargeable batteries, such as solid-state lithium metal batteries , and lithium–sulfur batteries. , Nevertheless, the formation of lithium dendrites during the charging and discharging processes poses a significant challenge. This phenomenon can potentially lead to separator penetration, causing short circuits and presenting safety hazards .…”
Section: Introductionmentioning
confidence: 99%