2022
DOI: 10.26434/chemrxiv-2022-scm3x
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Advantages and Limitations of Hydrogen Peroxide for Direct Oxidation of Methane to Methanol at Mono-Copper Active Sites in Cu-Exchanged Zeolites

Abstract: The oxidant is a crucial factor affecting the performance of direct oxidation of methane to methanol (DMTM). It is still extremely challenging to realize one-pot DMTM using dioxygen. So far, hydrogen peroxide is still the most frequently reported green oxidant for DMTM with high selectivity of methanol. Aiming to achieve insights into the influence of oxidants on the DMTM performance and to improve catalysts, we computationally investigated the reaction mechanisms of DMTM using hydrogen peroxide at mono-copper… Show more

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