Abstract. Vertical structures of aerosol single scattering albedo
(SSA), from near the surface through the free troposphere, have been
estimated for the first time at distinct geographical locations over the
Indian mainland and adjoining oceans, using in situ measurements of aerosol
scattering and absorption coefficients aboard the Facility for Airborne
Atmospheric Measurements (FAAM) BAe-146 aircraft
during the South West Asian Aerosol Monsoon Interactions (SWAAMI) campaign
from June to July 2016. These are used to examine the spatial variation of
SSA profiles and also to characterize its transformation from just prior to
the onset of Indian Summer Monsoon (June 2016) to its active phase (July
2016). Very strong aerosol absorption, with SSA values as low as 0.7,
persisted in the lower altitudes (<3 km) over the Indo-Gangetic
Plains (IGP), prior to the monsoon onset, with a west-to-east gradient;
lower values occurred in the north-western arid regions, peaking in the
central IGP and somewhat decreasing towards the eastern end. During the
active phase of the monsoon, the SSA is found to increase remarkably,
indicating far less absorption. Nevertheless, significant aerosol absorption
persisted in the lower and middle troposphere over the IGP. Inputting these
SSA and extinction profiles into a radiative transfer model, we examined the
effects of using height-resolved information in estimating atmospheric
heating rates due to aerosols, over similar estimates made using a single
columnar value. It was noted that use of a single SSA value leads to an
underestimation (overestimation) of the heating rates over regions with low
(high) SSA, emphasizing the importance of height-resolved information.
Further, the use of realistic profiles showed significant heating of the
atmosphere by submicron aerosol absorption at the middle troposphere, which
may have strong implications for clouds and climate.