Wearable sensors are vital for the development of electronic
skins
to improve health monitoring, robotic tactile sensing, and artificial
intelligence. Active materials and the construction of microstructures
in the sensitive layer are the dominating approaches to improve the
performance of pressure sensors. However, it is still a challenge
to simultaneously achieve a sensor with a high sensitivity and a wide
detection range. In this work, using three-dimensional (3D) vertical
graphene (VG) as an active material, in combination with micropyramid
arrays and lumpy holders, the stress concentration effects are generated
in nano-, micro-, and macroscales. Therefore, the lumpily pyramidal
VG film-based pressure sensor (LPV sensor) achieves an ultrahigh sensitivity
(131.36 kPa–1) and a wide response range (0.1–100
kPa). Finite element analysis demonstrates that the stress concentration
effects are enhanced by the micropyramid arrays and lumpy structures
in micro- and macroscales, respectively. Finally, the LPV pressure
sensors are tested in practical applications, including wearable health
monitoring and force feedback of robotic tactile sensing.