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INTRODUCTIONThe free-electron laser (FEL) sources FLASH in Hamburg, LCLS at Stanford and FERMI in Trieste provide XUV to soft x-ray radiation (FLASH and FERMI) or soft to hard x-ray radiation (LCLS) with unprecedented parameters in terms of ultrashort pulse length, high photon flux, and coherence. These properties make FELs ideal tools for studying ultrafast dynamics in matter on a previously unaccessible level. This paper reviews first results obtained at FEL sources during the last years in the field of magnetism research. We start with pioneering experiments at FLASH demonstrating the feasibility of magnetic scattering at FELs [1,2], then present pump-probe scattering experiments [3,4] as well as the first FEL magnetic imaging experiments [5], and finally discuss a limitation of the scattering methods due to a quenching of the magnetic scattering signal by high-fluence FEL pulses [6]. All of the presented experiments exploit the x-ray magnetic circular dichroism effect [7,8] to obtain element-specific magnetic scattering contrast, as known from synchrotron experiments [9][10][11][12].One of the key problems in modern magnetism research, ultrafast demagnetization discovered by Beaurepaire in 1996 [13], acts on time scales of a few 100 fs, which are not accessible at standard synchrotron radiation sources. Since its discovery, ultrafast demagnetization was studied using optical femtosecond lasers, for a review see e. g.[14], and femtoslicing sources [15] at storage ring sources [16,17]. In both cases, spatial resolution is limited due to wavelength or flux limitations. In contrast, FELs combine high time resolution, element selectivity, and the spatial resolving power of xrays with high photon flux and excellent coherence properties. FEL sources, therefore, promise a pivotal step forward in the investigation of ultrafast phenomena on nanometer length scales. The rapid development of the FELs with respect to even shorter pulses, increased pulse stability, and special double-pulse schemes, e. g. for ultrafast movies [18], will open up exciting new opportunities in the field of material science.
RESONANT SCATTERING FROM MAGNETIC DOMAIN SYSTEMSThe very first proof-of-principle resonant magnetic scattering experiment at x-ray FEL sources was carried out at FLASH in Hamburg [1]. In 2009 FLASH covered a photon energy range in the fundamental from 6.5 up to 50 nm with the routinely used cobalt L 3 -edge at 1.59 nm out of reach. However, by using the higher harmonics of the radiation 3 shorter wave length can be reached on the expense of photon flux. In this experiment FLASH was fine tuned to a fundamental wave length of 7.97 nm which results in the fifth harmonic located at the cobalt L 3 -edge. The scattering pattern from magnetic domains of a cobalt/palladium multilayer system with a perpendicular magnetic anisotropy and typical domain widths in the 100 nm range was recorded. This demonstrated that magnetic scattering as it is performed at synchrotron radiation sources is feasible at FELs. However, the fifth harmo...