According to the most recent Intergovernmental Panel on Climate Change (IPCC) report, the radiative forcing due to aerosols from observation-based evidence was assessed to be −0.4 ± 0.4 W m −2 (IPCC, 2021). This is likely able to offset part of the warming induced by the emission of greenhouse gases (Rosenfeld et al., 2019). However, the uncertainty remains of the same order as the estimated forcing.Whether aerosols directly warm or cool locally not only depends on aerosol physical and chemical properties, but also relies on the properties of the vertically overlapping clouds. Aerosols located above liquid clouds frequently occur off the west coast of continents as well as over the North Pacific and North Atlantic Oceans (Devasthale & Thomas, 2011). Strong reflection of liquid clouds enhances the above-cloud aerosol absorption, resulting in an increase of aerosol radiative heating rate and a change of the sign of net radiative effect at the top of atmosphere (TOA) (Chang & Christopher, 2017;Matus & L'Ecuyer, 2017;Meyer et al., 2013). For instance, biomass burning aerosols can switch from a net cooling to a net warming effect at the TOA with an increase of underlying cloud fraction (Chand et al., 2009;Keil & Haywood, 2003). Similarly, increase of underlying cloud fraction and optical depth was found to enhance the warming effect of dust aerosols (Xu et al., 2017). A cirrus layer above an aerosol layer is able to cause modest change of the radiative effect of absorbing or nonabsorbing aerosols at the TOA (Liao & Seinfeld, 1998). Considering the wide coverage of cirrus clouds and their strong regulation on the Earth's radiation (e.g., Hong & Liu, 2015;Hong et al., 2016), cirrus impact on aerosol direct radiative effect could be extraordinary, which by now has not been assessed over the globe.Incomplete knowledge of aerosol-cloud interactions also challenges an accurate estimate of the direct radiative effect of aerosols. Cloud active aerosols interact with clouds by modifying cloud microstructure such as reducing liquid cloud effective radius (