In this Letter, two comparator-based voltage-mode hysteretic controller designs are proposed to enhance dynamic response for single-inductor multiple-output (SIMO) switching converters to minimise over-/ under-shoot voltages due to self-and cross-regulations in fast load transients, especially with high output power and large current steps. The proposed converters are designed and simulated in a 65 nm CMOS process with standard I/O devices. With the proposed techniques, the output voltage fluctuations, including steady-state voltage ripples and over-/under-shoot voltages due to self-and crossregulations during a 1.8 A load transient in 1 ns, are kept within 60 mV. The proposed converter delivers more than 3 A maximum load current per output and a maximum total output power above 6 W, with a peak efficiency above 90%. Compared to state-of-the-art SIMO converters, this work achieves a significantly higher output power capacity and faster dynamic response thus smaller self-and cross-regulations within 0.033 mV/mA.