An active learning approach to model solid-electrolyte interphase formation in Li-ion batteries

Soleymanibrojeni, Mohammad; Caldeira Rego, Celso Ricardo; Esmaeilpour, Meysam; Wenzel, Wolfgang

doi:10.1039/d3ta06054c

J. Mater. Chem. A

2024

DOI: 10.1039/d3ta06054c

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An active learning approach to model solid-electrolyte interphase formation in Li-ion batteries

Mohammad Soleymanibrojeni,

Celso Ricardo Caldeira Rego,

Meysam Esmaeilpour

et al.

Abstract: Li-ion batteries store electrical energy by electrochemically reducing Li ions from a liquid electrolyte into a graphitic electrode. During these reactions, electrolytic species in contact with the electrode particles form...

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A review of recent developments in the design of electrolytes and solid electrolyte interphase for lithium metal batteries

Kang,

Lyu

et al. 2024

EcoMat

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Lithium metal batteries offer a promising solution for high density energy storage due to their high theoretical capacity and negative electrochemical potential. However, implementing of these batteries faces challenges related to electrolyte instability and the formation of a solid electrolyte interphase (SEI) on the lithium (Li) metal anode. The decomposition of liquid electrolytes leading to the creation of the SEI emphasizes the significance of the type of Li salt, solvent, and additives designed and used, as well as their interactions during the formation of the SEI. For practical applications, ensuring both the reversibility of the Li metal anode and electrolyte stability at high voltages is crucial. In this review, we explore recent advancements in addressing these challenges through new designs of electrolytes and SEI engineering practices. Specifically, we investigate the effects of electrolyte systems, including carbonate‐based and ether‐based solutions, along with modifications to these electrolyte systems aimed at achieving a more stable interface with the Li metal anode. Additionally, we discuss various artificial SEI structures based on organic and inorganic components. By critically examining recent research in these areas, this review provides valuable insights into current state‐of‐the‐art strategies for enhancing the performance and safety of Li metal batteries.image

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A review of recent developments in the design of electrolytes and solid electrolyte interphase for lithium metal batteries

Kang,

Lyu

et al. 2024

EcoMat

View full text Add to dashboard Cite

show abstract

Recent advances in artificial intelligence boosting materials design for electrochemical energy storage

Liu,

Fan,

Huang

et al. 2024

Chemical Engineering Journal

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An active learning approach to model solid-electrolyte interphase formation in Li-ion batteries

Abstract: Li-ion batteries store electrical energy by electrochemically reducing Li ions from a liquid electrolyte into a graphitic electrode. During these reactions, electrolytic species in contact with the electrode particles form...

Cited by 2 publications

References 29 publications

A review of recent developments in the design of electrolytes and solid electrolyte interphase for lithium metal batteries

A review of recent developments in the design of electrolytes and solid electrolyte interphase for lithium metal batteries

Recent advances in artificial intelligence boosting materials design for electrochemical energy storage

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