Over the last decade, spatially-explicit modeling of landscape-scale forest attributes for forest inventories has greatly benefitted from airborne laser scanning (ALS) and the area-based approach (ABA) to derive wall-to-wall maps of these forest attributes. Which ALS-derived metrics to include when modeling forest inventory attributes, and how prediction accuracies vary over forest types depends largely on the structural complexity of the forest(s) being studied. Hence, the purpose of this study was to (i) examine the usefulness of adding texture and intensity metrics to height-based ALS metrics for the prediction of several forest resource inventory (FRI) attributes in one boreal and two Great Lakes, St. Lawrence (GLSL) forest region sites in Ontario and (ii) quantify and compare the site and forest type variability within the context of the FRI prediction accuracies. Basal area (BA), quadratic mean diameter-at-breast height (QMD), and stem density (S) were predicted using the ABA and a nonparametric Random Forests (RF) regression model. At the site level, prediction accuracies (i.e., expressed as RMSE (Root Mean Square Error), bias, and R2) improved at the three sites when texture and intensity metrics were included in the predictor set, even though no significant differences (p > 0.05) could be detected using the nonparametric RMANOVA test. Stem density benefitted the most from the inclusion of texture and intensity, particularly in the GLSL sites (% RMSE improved up to 6%). Combining site and forest type results indicated that improvements in site level predictions, due to the addition of texture and intensity metrics to the ALS predictor set, were the result of changes in prediction accuracy in some but not all forest types present at a site and that these changes in prediction accuracy were site and FRI attribute specific. The nonparametric Kruskal–Wallis test indicated that prediction errors between the different forest types were significantly different (p ≤ 0.01). In the boreal site, prediction accuracies for conifer forest types were higher than for deciduous and mixedwoods. Such patterns in prediction accuracy among forest types and FRI attributes could not be observed in the GLSL sites. In the Petawawa Research Forest (PRF), we did detect the impact of silvicultural treatments especially on QMD and S predictions.