In this paper, we reviewed the existing literature on the fabrication of nanocomposites based on cellulose and cellulose nanocrystals (CNCs), and analyzed their dispersion mechanism with respect to their use in the field of construction. First, the existing literature on CNC-based nanocomposites that exhibit the physical and chemical properties of nanocellulose and CNCs was reviewed. Next, keeping the use of these nanocomposites in the field of construction in mind, we determined the optimal mechanical method for their dispersion as an alternative to the currently used harmful chemical techniques. To this end, we evaluated the dispersibility of colloidal CNCs using two dispersion methods: magnetic stirring (for stirring times of 60 min, 120 min, and 180 min) and high-pressure dispersion (at pressures of 345 × 10 5 Pa, 1035 × 105 Pa, and 1587 × 10 5 Pa, and one to three dispersion passes). The optimal dispersion conditions were determined by analyzing the size and zeta potential of the CNC particles. It was found that the difference in the average diameter was reduced by approximately 76% at 1587 × 10 5 Pa during high-pressure dispersion. modulus of 200-220 GPa, density of approximately 8 g/cm 3 .) While the process for producing CNCs is a complex one, the final product suggests improvements in the cement composites by improving mechanical properties. Calcium silicate hydrate (CSH) gel formation was improved in CNC cement mortar, with the compressive strength of the mortar being 42-45% higher than that of conventional cement mortar. The formation of the CSH gel improved the strength of the cement by improving its hydration. In order to quantify the performance of cement composites based on CNCs, their degree of hydration was measured using an isothermal calorimeter and a thermogravimetric analyzer [18,19].Studies on the application of cement to conventional CNCs have been carried out only in some strength studies using optimal mixing conditions. Ultrasonic methods are primarily used to disperse CNCs [16,[18][19][20][21]. However, ultrasonic dispersion techniques have certain limitations with respect to the production of cement paste and mortar, because they can only produce small amounts of CNC suspensions (10-250 mL by Sonics and Processor USA). When attempting to produce large amounts of CNC suspensions, as is the case when making concrete mixtures, the ultrasonic dispersion equipment may exhibit problems caused by prolonged use.Therefore, methods should be developed that allow one to prepare CNC-based concrete on a large scale while causing fewer equipment problems. In this study, we attempted to determine the optimal CNC dispersion conditions based on an evaluation of the previously reported dispersion data with the aim of using CNCs as a construction material.
Review of Existing ResearchWe reviewed previous studies on cellulose and cellulose nanomaterials that are relevant to the field of construction. Table 1 summarizes the review of the existing literature on CNCs.