In slope ecological restoration projects, reinforcing soil and promoting vegetation growth are essential measures. Guest soil spraying technology can be used to backfill modified soil and vegetation seeds onto the slope surface, resulting in successful ecological restoration. The use of organic polymer modifiers to reinforce soil has several benefits, such as high strength, effective results, and low pollution levels. Organic polymer soil modifiers can be divided into two categories: synthetic polymer modifiers and biopolymer modifiers. This paper provides a thorough review of the properties and interaction mechanisms of two types of polymer modifiers in soil consolidation. The properties of organic polymer modifiers make them applicable in soil and vegetation engineering on slopes. These modifiers can enhance soil mechanics, infiltration, and erosion resistance and promote vegetation growth. Therefore, the suitability of organic polymer modifiers for soil and vegetation engineering on slopes is demonstrated by their properties and potential for improvement in key areas. Furthermore, challenges and future prospects for slope protection technology using organic polymer modifiers are suggested.