Abaca fibres that have excellent mechanical properties are widely applied in the production and preparation of eco-friendly polymer composites as reinforcement materials. However, the weak interfacial bonding property of the abaca fibre and composite matrix limits the further extended application of abaca fibre-reinforced polymer composites. In this research, the findings demonstrate that, compared to raw abaca fibres, the interfacial shear strength (IFSS) value between the treated fibre and matrix is improved by 32% to 86%. Moreover, chemically treated abaca fibres could not only improve the wear resistance of the polymer composites, but also could promote the formation of primary and secondary plateaus. The best wear resistance behaviour was demonstrated by the sample with abaca fibres treated with 3% NaOH and 5% silane solutions, which had a maximum reduction in the sum wear rate of 28.44%. This research will provide detail on theoretical guidance and technical support for the development of eco-friendly natural fibre-reinforced polymer composites.