An experimental study on carbon dioxide hydrate formation using a gas-inducing agitated reactor

Li, Airong; Jiang, Lele; Tang, Siyao

doi:10.1016/j.energy.2017.06.023

Cited by 55 publications

(32 citation statements)

References 28 publications

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“…Various ‘agitated reactors’ with a stirred‐vessel configuration for better hydrate conversion have been presented in the literature . They improved gas / water contact and, as a result, the gas uptake during hydrate formation increased significantly.…”

Section: Hydrate‐based Co2 Capture and Separation Technologymentioning

confidence: 99%

“…A high gas uptake and separation factor could be achieved through mechanical agitation to renew the contact surface area continuously. In our laboratory, we also investigated a series of experiments on CO 2 hydrate formation, which was efficiently enhanced through mechanical agitation and gas recycling . However, the power consumption associated with mechanical agitation is too high, raising the cost again, which makes it infeasible to scale up the large industrial separation.…”

Section: Hydrate‐based Co2 Capture and Separation Technologymentioning

confidence: 99%

“…Various 'agitated reactors' with a stirred-vessel configuration for better hydrate conversion have been presented in the literature. 32,40,99 They improved gas / water contact and, as a result, the gas uptake during hydrate formation increased significantly. An agitated gas-inducing crystallizer was reported by Linga et al 40 A high gas uptake and separation factor could be achieved through mechanical agitation to renew the contact surface area continuously.…”

Section: Hydrate Formation Reactorsmentioning

confidence: 99%

“…In our laboratory, we also investigated a series of experiments on CO 2 hydrate formation, which was efficiently enhanced through mechanical agitation and gas recycling. 99 However, the power consumption associated with mechanical agitation is too high, raising the cost again, which makes it infeasible to scale up the large industrial separation. From the equipment design perspective, the proper use of a high-pressure flue gas stream to produce the agitation could mitigate the power input, taking into account that flue gas itself is a feeding stream in hydrate formation.…”

Section: Hydrate Formation Reactorsmentioning

confidence: 99%

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High‐efficiency CO₂ capture and separation based on hydrate technology: A review

Wang

Bao

2019

Greenhouse Gases

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As a result of growing concerns about global warming, hydrate‐based processing is becoming a promising technology for CO2 capture. This process captures CO2 by forming clathrate hydrates by exposing flue gas to water under suitable conditions. It results in high CO2 recovery due to its large gas‐storage capacity and the large concentration differences between the separation phases. However, the high cost of hydrate formation conditions is the main reason preventing this technology from wide industrial application. To address this issue, this paper explores the literature on the current status of developments in hydrate‐based CO2 capture and separation, focusing on methods to mitigate hydrate formation conditions and to improve phase‐contacting performance. In this review, various relevant aspects of CO2 capture and separation selectivity are summarized, including promoter selection, thermodynamic and kinetic model development, reactor configuration, and process design. Advantages and disadvantages of alternative processes are also discussed. Current studies are limited to laboratory experiments but low energy penalties and high CO2 selectivity features of hydrate processes will make future plant implementation feasible. © 2019 Society of Chemical Industry and John Wiley & Sons, Ltd.

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Section: Hydrate‐based Co2 Capture and Separation Technologymentioning

confidence: 99%

Section: Hydrate‐based Co2 Capture and Separation Technologymentioning

confidence: 99%

Section: Hydrate Formation Reactorsmentioning

confidence: 99%

Section: Hydrate Formation Reactorsmentioning

confidence: 99%

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High‐efficiency CO₂ capture and separation based on hydrate technology: A review

Wang

Bao

2019

Greenhouse Gases

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“…A correlation was also used to calculate the order of nucleation [18]. Li et al (2017) investigated carbon dioxide hydrate formation using a gasinducing agitated reactor. The results showed that the induction time was greatly shortened from 261 to 24 min as the rotation speed increased from 0 to 800 rpm.…”

Section: Introductionmentioning

confidence: 99%

Effect of TBAB and SDS surfactants on the interfacial tension of CO2 Hydrate in water

2020

Eurasian Chem. Commun.

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The interfacial tension rate is an important factor in the kinetic study of gas hydrate formation. In this study, the interfacial tension between CO2 hydrate and water was calculated at various temperatures, pressures and solution concentrations through measuring the induction time according to the Classical Nucleation Theory (CNT). Since the nucleation of hydrate is in part an interfacial phenomenon, interfacial properties such as the interfacial tension between gas and water may have a great influence upon the hydrate formation rate. Experimental data for pure water showed that, at constant temperature, with increasing pressure, the interfacial tension decreases from 2.92 to 1.67 mN/m, and at constant pressure with increasing temperature, interfacial tension increases from 3.92 to 4.7 mN/m. At constant temperature, with increasing TBAB concentration from 1% to 3% by weight, the induction time decreases from 60 to 36 seconds. At higher temperatures, addition of SDS 500 ppm decreased the induction time and interfacial tension from 4.61 to 2.32 m N/m. Finally, the relationship of nucleation intensity with the super saturation was obtained by fitting the experimental data. According to equations and graphs, the nucleation intensity is a function of temperature.

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Modeling of CO ₂ storage as hydrate in vacated natural gas hydrate formation

Ahmad

et al. 2019

Int J Energy Res

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An experimental study on carbon dioxide hydrate formation using a gas-inducing agitated reactor

Cited by 55 publications

References 28 publications

High‐efficiency CO₂ capture and separation based on hydrate technology: A review

High‐efficiency CO₂ capture and separation based on hydrate technology: A review

Effect of TBAB and SDS surfactants on the interfacial tension of CO2 Hydrate in water

Modeling of CO ₂ storage as hydrate in vacated natural gas hydrate formation

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An experimental study on carbon dioxide hydrate formation using a gas-inducing agitated reactor

Cited by 55 publications

References 28 publications

High‐efficiency CO2 capture and separation based on hydrate technology: A review

High‐efficiency CO2 capture and separation based on hydrate technology: A review

Effect of TBAB and SDS surfactants on the interfacial tension of CO2 Hydrate in water

Modeling of CO 2 storage as hydrate in vacated natural gas hydrate formation

Contact Info

Product

Resources

About

High‐efficiency CO₂ capture and separation based on hydrate technology: A review

High‐efficiency CO₂ capture and separation based on hydrate technology: A review

Modeling of CO ₂ storage as hydrate in vacated natural gas hydrate formation