This work is the result of efforts by many people, both in a professional and a personal sense. During my time in Berkeley I had the opportunity to work with friendly and supportive people who were pushing back scientific boundaries, regarding the limits of superconducting high field technology. It is an odd but good experience to read papers from various authors detailing one scientific breakthrough or another, and then to meet them in person. Being a multi-cultural hub, Berkeley also allowed me to meet and become friends with people from all corners of this planet.Along the way, people have been instrumental in making this research happen. At LBNL, Jonathan Slack, Reuben Mendelsberg, and Andre Anders allowed me to use their lab for a rather extended period of time thus allowing for the fabrication of thin films, and have helped in various other ways along the years. The people at Ohio State University have helped by repeatedly performing heat capacity measurements on Nb 3 Sn bulk samples which were kindly supplied by Wilfried Goldacker of the Karlsruhe Institute of Technology. In particular I would like to thank Mike Susner of the Ohio State University, who came to the lab in the weekends just to make sure my samples would get measured. John Bonevich of the National Institute of Science and Technology was kind enough to perform characterization work on some of the Nb-Sn thin films we made, which included the STEM image on the cover. A lot of the experimental work was made possible with software and hardware designed at the University of Twente (such as VI by Bennie ten Haken), and I have gotten useful recommendations and assistance along the way, such as the advice on thin film fabrication from Frank Roesthuis. Professors Marcel ter Brake, Herman ten Kate, David Larbalestier, and Frances Hellman were kind enough to write letters of recommendation which contributed to getting the CSC student fellowship award. Vladimir Kresin of LBNL was kind enough to answer various questions related to the microscopic properties of Nb 3 Sn and comment on the description of microscopic theory in this thesis.Shane Cybart and Stephen Wu have assisted Edwin Dollekamp and myself in attempting to do some very fancy experiments. Edwin, from the University of Twente, took on a complicated research topic and I was impressed with how far he managed to get in that work, and Shane and Stephen invested time in the evenings and weekends to make it happen. Professor Orlandos previous investigations of Nb 3 Sn were an inspiration for some of the work described in this thesis, and he was kind enough to answer questions by email and over the phone. Derek Stewart of the Cornell NanoScale Science and Technology Facility helped me to get familiar with density functional theory calculations and computing clusters and made the suggestion of using Quantum Espresso ab-initio software. Robert Ryne and Steve Gourlay of LBNL helped me getting access to sizeable supercomputing resources at NERSC which were needed for this research.My friends and family st...