Naturally occurring radionuclide activity was investigated at landfill sites from the City of Cape Town using a Hyper-Pure Geranium detector with appropriate shielding coupled to a Palmtop Multichannel Analyzer. Activity concentrations of the radionuclides 238 U, 232 Th and 40 K were obtained from the activity concentrations of their respective daughter radionuclides. To obtain the overall combined effect in terms of activity concentration from the 3 parent radionuclides, the radium equivalent was calculated and 38.273, 41.019 and 83.007 Bq/Kg were obtained from Bellville, Coastal Park, and Vissershok respectively. Other radiological hazards in terms of Internal and External hazard indices and Representative hazard index were determined and found to be within safe limits. Dose rate in air at 1m above the ground was determined to obtain a characteristic of the external gamma-ray and was found to be 17.490, 18.609 and 38.667 nGy/y for Bellville, Coastal Park, and Vissershok respectively. The health effects of the radiation in terms of annual effective dose and excess lifetime cancer risk were determined to be 0.031 mSv/y and 0.0961×10 -3 which are lower than limits set by the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) and the Nuclear Industry Association of South Africa (NIASA).