Piezoelectric flags have functions of both classic flags and energy harvesting, and are becoming a new research focus. Interface circuits that convert wind energy to electrical energy are the key component of piezoelectric flags. A new structure for piezoelectric flags was designed to generate vibration by wind induction. After theoretical analysis, only SEH (standard energy harvesting) and SSHC (synchronized switch-harvesting-on capacitors) interface circuits were found suitable for piezoelectric flags. Simulation in Multisim was performed to compare SEH and SSHC in different load resistance. Experiments were carried out using different wind speeds. The on-time and delay-time of each switch were controlled by the proposed control algorithm. Both simulation and experimental results indicate that the output voltage with SSHC is higher than the output voltage with SEH. When the resistance is 1700 kΩ and the wind speed is 24 m/s, the output power of SSHC can be increased by 45.63% compared with the SEH circuit.