2017
DOI: 10.1002/adfm.201700264
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An Ultrahigh Responsivity (9.7 mA W−1) Self‐Powered Solar‐Blind Photodetector Based on Individual ZnO–Ga2O3 Heterostructures

Abstract: Highly crystallized ZnO–Ga2O3 core–shell heterostructure microwire is synthesized by a simple one‐step chemical vapor deposition method, and constructed into a self‐powered solar‐blind (200–280 nm) photodetector with a sharp cutoff wavelength at 266 nm. The device shows an ultrahigh responsivity (9.7 mA W−1) at 251 nm with a high UV/visible rejection ratio (R251 nm/R400 nm) of 6.9 × 102 under zero bias. The self‐powered device has a fast response speed with rise time shorter than 100 µs and decay time of 900 µ… Show more

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Cited by 698 publications
(292 citation statements)
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References 51 publications
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“…Besides, BN based PDs begin to attract substantial attentions for solar-blind detection [102][103][104] due to a wide bandgap of 5.2 eV (hexagonal BN) or 6.4 eV (cubic BN). 116) In addition, groups of novel materials including ZnO, 105,106) Ga 2 O 3 , 107-109) MgZnO, [110][111][112] and two-dimensional (2D) perovskite 113) and nanostructures in the form of superlattice (SL), 103) nanowires (NWs), core-shell structures 109) have emerged thanks to the advances in material growth and fabrication techniques. The transient response, or stability of these novel solar-blind PDs still requires further investigation, and implementation of these devices in communication are still lacking.…”
Section: Detectorsmentioning
confidence: 99%
See 1 more Smart Citation
“…Besides, BN based PDs begin to attract substantial attentions for solar-blind detection [102][103][104] due to a wide bandgap of 5.2 eV (hexagonal BN) or 6.4 eV (cubic BN). 116) In addition, groups of novel materials including ZnO, 105,106) Ga 2 O 3 , 107-109) MgZnO, [110][111][112] and two-dimensional (2D) perovskite 113) and nanostructures in the form of superlattice (SL), 103) nanowires (NWs), core-shell structures 109) have emerged thanks to the advances in material growth and fabrication techniques. The transient response, or stability of these novel solar-blind PDs still requires further investigation, and implementation of these devices in communication are still lacking.…”
Section: Detectorsmentioning
confidence: 99%
“…Table II summarizes the performance of semiconductor based solar-blind PDs. 88,[96][97][98][99][100][101][102][103][104][105][106][107][108][109][110][111][112][113] The table is ordered by the use of different groups of materials. As indicated in the table, III-nitride based PDs are among the first and ideal choices for high efficiency and high-speed devices.…”
Section: Detectorsmentioning
confidence: 99%
“…[1][2][3][4][5][6][7][8][9][10][11][12][13][14] Here, a sol-gel method has been developed and used for the fabrication of (relatively) thick porous polycrystalline ZnO layers. A similar method has already been reported for thin films by, e.g., Gohdsi et al 34 and Choudhury et al 44 Here the method has been extended for obtaining well-defined thick ZnO films (up to ∼2 μm) by using a sequential drop-cast approach in a 'vacuum' environment.…”
Section: 2mentioning
confidence: 99%
“…1,2 ZnO has been studied extensively as a candidate for a number of applications, e.g., transparent conductive electrodes, optical waveguides, piezo-electric transducers, acoustic wave devices, conductive gas sensors, solar cell windows and biosensing. [1][2][3][4][5][6][7][8][9][10][11][12][13][14] This makes it attractive for the fields of optoelectronics, 2,15,16 sensors, 1,5 piezoelectrics 7,17 and biomedical applications. 8 In addition, nanostructured ZnO coatings can provide new ways for light manipulation (e.g.…”
mentioning
confidence: 99%
“…The response time (t r ) and decay time (t d ) are defined as the duration for photocurrent to rise from 10% to 90% of the peak value and to decrease from 90% to 10% of the peak value, respectively. 29 An enlarged view of the rise and decay processes of the photovoltage under 532 nm modulated laser (10 Hz) is shown in Fig. 4(c).…”
mentioning
confidence: 99%