Catapult-assisted takeoff is the initiation of flight missions for carrier-based aircrafts. Ensuring the safety of aircrafts during catapult-assisted takeoff requires a thorough analysis of their motion characteristics. In this paper, a rigid–flexible coupling model using the Finite Element Method and Multibody Dynamics (FEM-MBD) approach is developed to simulate the aircraft catapult process. This model encompasses the aircraft frame, landing gear, carrier deck, and catapult launch system. Firstly, reasonable assumptions were made for the dynamic modeling of catapult-assisted takeoff. An enhanced plasticity algorithm that includes transverse shear effects was employed to simulate the tensioning and release processes of the holdback system. Additionally, the forces applied by the launch bar and holdback bar, nonlinear aerodynamics loads, shock absorbers, and tires were introduced. Finally, a comparative analysis was conducted to assess the influence of different launch bar angles and holdback bar fracture stain on the aircraft’s attitude and landing gear dynamics during the catapult process. The proposed rigid–flexible coupling dynamics model enables an effective analysis of the dynamic behavior throughout the entire catapult process, including both the holdback bar tensioning and release, takeoff taxing, and extension of the nose landing gear phases. The results show that higher launch bar angle increase the load and extension of the nose landing gear and cause pronounced fluctuations in the aircraft’s pitch attitude. Additionally, the holdback bar fracture strain has a significant impact on the pitch angle during the first second of the aircraft catapult process, with greater holdback bar fracture strain resulting in larger pitch angle variations.