“…Despite appreciable development of optoelectronics in recent years, many problems related to semiconductor processing and the efficiency of the devices are still unresolved. Therefore, new stable, processable organic compounds that are able to meet the continually increasing demands are being sought. − Among the various π-conjugated compounds, azomethines have attracted broad research interest as components in optoelectronic devices. − Imines are synthesized under mild reaction conditions, where only water is formed as a byproduct (the reaction is not harmful to the environment), and do not require a complicated purification process and metal catalysts. − , The possibility of modification of the azomethine structure through the appropriate selection of amines and carbonyl compounds allows for the preparation of new compounds with the desired properties. Considering the chemical structure of the investigated imines for organic electronics, special attention is paid to heterocyclic azomethines with a thiophene unit. − Compounds with a thiophene structure exhibit many desirable properties in optoelectronics, such as low oxidation potentials, low band-gap energy, good electrical conductivity, and chemical and thermal stability. ,− ,, Apart from the various fields of imine applications, they are also investigated as materials for photovoltaic (PV) cells. − Nowadays, they are examined in bulk heterojunctions (BHJs), − dye-sensitized solar cells (DSSCs), and perovskite solar cells (PSCs).…”