“…To address these questions, our first challenge is to distinguish reliable from unreliable trajectory statistics. Ultimately, trajectories should be validated with predictions of constituent concentrations that can be verified with satellite and aircraft data [e.g., Fueglistaler et al, 2005;James et al, 2008;Ploeger et al, 2011;Bergman et al, 2014;Ueyama et al, 2014;Jensen et al, 2015]. However, these predictions require knowledge of the constituent sources and process models that alter concentrations along the trajectories.…”