Anti-solvent engineering enables efficient ambient-processed halide perovskite solar cells

Asuo, Ivy M.; Mahdavi Varposhti, Arezo; Gomez, Enrique D.; Doumon, Nutifafa Y.

doi:10.1039/d4tc01305k

J. Mater. Chem. C

2024

DOI: 10.1039/d4tc01305k

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Anti-solvent engineering enables efficient ambient-processed halide perovskite solar cells

Ivy M. Asuo,

Arezo Mahdavi Varposhti,

Enrique D. Gomez

et al.

Abstract: Organic-inorganic metal halide perovskite thin film formation is one of the major challenges for solution-processed perovskite optoelectronic and photovoltaic devices, in particular, in ambient due to their hygroscopic nature. Therefore,...

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Cited by 3 publications

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Metal–Organic Frameworks and Derivative Materials in Perovskite Solar Cells: Recent Advances, Emerging Trends, and Perspectives

Shah,

Sayyad,

Guo

2024

Solar RRL

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The power conversion efficiency (PCE) of perovskite solar cells (PSCs) has reached an impressive value of 26.1%. While several initiatives such as structural modification and fabrication techniques helped steadily increase the PCE and stability of PSCs in recent years, the incorporation of metal–organic frameworks (MOFs) in PSCs stands out among other innovations and has emerged as a promising path forward to make this technology the front‐runner for realizing next‐generation low‐cost photovoltaic technologies. Owing to their unique physiochemical properties and extraordinary advantages such as large specific surface area and tunable pore structures, incorporating them as/in different functional layers of PSCs endows the devices with extraordinary optoelectronic properties. This article reviews the latest research practices adapted in integrating MOFs and derivative materials into the constituent blocks of PSCs such as photoactive perovskite absorber, electron‐transport layer, hole‐transport layer, and interfacial layer. Notably, a special emphasis is placed on the aspect of stability improvement in PSCs by incorporating MOFs and derivative materials. Also, the potential of MOFs as lead absorbents in PSCs is highlighted. Finally, an outlook on the critical challenges faced and future perspectives for employing MOFs in PSCs in light of the commercialization of PSCs is provided.

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Metal–Organic Frameworks and Derivative Materials in Perovskite Solar Cells: Recent Advances, Emerging Trends, and Perspectives

Shah,

Sayyad,

Guo

2024

Solar RRL

View full text Add to dashboard Cite

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Light‐Emitting Perovskite Solar Cells: Genesis to Recent Drifts

Shah,

Sayyad,

Guo

2024

Solar RRL

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Perovskite, a star material with extraordinary opto‐electronic properties has shown promising results in both perovskite solar cells (PSCs) and perovskite light‐emitting diodes (PeLEDs). Taking advantage of the similar configuration of PSCs and PeLEDs, next generation devices with dual functionality of light‐harvesting and light‐emission can be realized. Such devices hold enormous application prospects. However, the necessary tradeoff resulted from the opposite working principles required for each mode of operation and challenges such as non‐radiative recombination loss resulted from bulk and surface defects in perovskite films and mismatched energy levels have hindered mass production. To provide a roadmap for rationally designing efficient light emitting perovskite solar cells (LEPSCs), a comprehensive review focusing on operating principle, device architecture, recent developments and limitations is required. We begin with a brief overview of the basic principles underlying the working mechanism of LEPSCs such as photon to electricity conversion and viceversa. The focus of this review then shift towards deligently combining and overviewing the important breakthroughs reported in this newly developed field such as morphology optimization, defect passivation, interface engineering, energy level alignment and dimensional control. Finally, this work concludes with discussing future challenges and providing a roadmap for rational design of efficient and stable LEPSCs.

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Semitransparent organic and perovskite photovoltaics for agrivoltaic applications

Kim,

Rayes,

Kemanian

et al. 2025

Energy Adv.

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Anti-solvent engineering enables efficient ambient-processed halide perovskite solar cells

Abstract: Organic-inorganic metal halide perovskite thin film formation is one of the major challenges for solution-processed perovskite optoelectronic and photovoltaic devices, in particular, in ambient due to their hygroscopic nature. Therefore,...

Cited by 3 publications

References 50 publications

Metal–Organic Frameworks and Derivative Materials in Perovskite Solar Cells: Recent Advances, Emerging Trends, and Perspectives

Metal–Organic Frameworks and Derivative Materials in Perovskite Solar Cells: Recent Advances, Emerging Trends, and Perspectives

Light‐Emitting Perovskite Solar Cells: Genesis to Recent Drifts

Semitransparent organic and perovskite photovoltaics for agrivoltaic applications

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