“…Since the 1960s, geochemical signals preceding significant earthquakes have been used for earthquake prediction, especially in China, Japan, the former Soviet Union, and the United States (KING, 1986;THOMAS, 1988). Gas monitoring on hydrothermal systems and fault zones has been prevailing because gas moves at a relatively high velocity within these areas (TAKAHATA et al, 1997;TOUTAIN and BAUBRON, 1999;WHITEHEAD and LYON, 1999;HEINICKE and KOCH, 2000). Changes in gas compositions (H 2 , CH 4 , CO 2 , and noble gases, especially Rn and He), and He/Ar, CH 4 /Ar, N 2 /Ar, and 3 He/ 4 He ratios, were reported to be potential precursors (KING, 1978;SUGISAKI, 1978;KAWABE, 1984;SUGISAKI and SUGIURA, 1986;IGARASHI et al, 1995;SANO et al, 1998;FYTIKAS et al, 1999;TEDESCO and SCARSI, 1999;ITALIANO et al, 2001;VIRK et al, 2001;CHYI et al, 2001CHYI et al, , 2005WALIA et al, 2005;.…”