Abstract. Deforestation for farming and grazing purposes has become a global challenge. To study the impact of deforestation on soil erosion rates and soil physicochemical properties, Zarivar Lake watershed, Kurdestan Province, Iran, was selected. Converting the steep hillslopes naturally under oak forest to rainfed vineyards has been one of the most common land-use changes in the area. We used 137Cs and 210Pbex radionuclides and quantified the Chernobyl-derived 137Cs fallout with 239+240Pu. The soil samples were collected from two adjacent and similar hillslopes, one of which is under natural forest, while the other is under rainfed vineyard. Using 137Cs/239+240Pu rates and a simple unmixing of the 137Cs sources indicated that 50.2 ± 10.0 % of 137Cs was Chernobyl-derived. The mean reference inventory values of 137Cs, 210Pbex, and 239+240Pu were estimated to be at 6152 ± 1266, 6079 ± 1511, and 135 ± 31 Bq m−2, respectively. At the forested hillslope, net soil erosion rates based on 137Cs, and 210Pbex, techniques were estimated to be at 5.0 and 5.9 Mg ha−1 yr−1, respectively, resulting in Sediment Delivery Ratios (SDRs) of 96 and 70 %. However, at the vineyard hillslope, the net soil redistribution rates were at 25.9 and 32.5 Mg ha−1 yr−1 for 137Cs and 210Pbex, respectively, resulting in respective SDRs of around 95 and 92 %. Both 137Cs and 210Pbex indicated that as a result of deforestation, soil erosion has increased by approximately five times. Percolation Stabilities (PS) in forest and vineyard topsoil are about 309 and 160 gr H2O 600 s−1 classified as rapid and moderate PSs, respectively. Rapid PS in forest soil implies high aggregate stability, whereas moderate PS in vineyard soils indicates that they are generally weakly-structured. All in all, the results of the present study revealed that deforestation and converting natural vegetation to cropland prompted soil loss and deteriorated physicochemical properties of the soil.