2024
DOI: 10.1021/acs.jpcc.3c08137
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Application of KR3F10 (R = Gd–Lu and Y) Polymorphism for Modeling the Defect Structure of Nonstoichiometric Multicomponent Fluorite-Type Crystals in T-x Systems

Elena A. Sulyanova,
Boris P. Sobolev

Abstract: Nonstoichiometric nanostructured crystals (NSC) α-M 0.5−x R 0.5+x F 2+2x (M = Na and K; R = Sc, Y, and La−Lu) and M 1−x R x F 2+x (M = Ca, Sr, Ba, Cd, and Pb) with a f luorite-type (F) structure are widely used in quantum electronics, optics, solid-state ionics (superionic conductors), and bioimaging. However, the temperature dependence of their defect crystal structure, which is fundamental for understanding the numerous properties of F-NSC, remains unexplored. In this study, temperature changes in the F-NSC … Show more

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