Application of MOF-derived materials as electrocatalysts for CO₂ conversion

Abstract

Electrochemical reduction CO2 into fuel/high-value chemicals using electricity generated from renewable energy is one of the most promising ways to achieve carbon neutrality. Recently, metal-organic frameworks (MOFs) derived materials, originating...

High-performance artificial leaf: from electrocatalyst design to solar-to-chemical conversion

“…29,30 In order to mitigate the increasing greenhouse effect and achieve the global zero-carbon goal, the development of efficient ways to reduce CO 2 to high value-added chemicals is important for both scientific research and practical applications. 31–35…”

Advances and challenges in the electrochemical reduction of carbon dioxide

“…245,246 MOFs are superb catalyst templates due to their outstanding physiochemical stability, structure diversity, highly ordered porous structure, uniform pore sizes and environments, high internal surface areas, and functional organic linkers. 247,248 Beneting from these unique physical and chemical properties, MOF derivatives exhibit the superiorities of higher stability, conductivity, and catalytic activity, which have been widely applied in CO 2 RR.…”

Metal‐Organic Frameworks‐Derived Nanocarbon Materials and Nanometal Oxides for Photocatalytic Applications

“…[56] Additionally, due to the advantageous properties of conductivity and stability in MOFsderived nanomaterials, they find applications as electrode materials in batteries or capacitors, [57] including the use of MOFs-derived nanomaterials in electrocatalysis and electrochemical sensors. [58,59] Additionally, MOFs-derived nanomaterials are also widely used in the field of photocatalysis. For example, Behera et al [60] has summarized the detailed preparation strategies of MOFs-derived nanomaterials, including thermal treatment, reflux synthesis method, chemical treatment method, and electrochemical fabrication method.…”

“…In previously reported review, MOFs‐derived nanomaterials have been recognized for their characteristics such as ease of modification, biocompatibility, and biodegradability, making them suitable for applications in antimicrobial materials for pharmaceuticals and food packaging [56] . Additionally, due to the advantageous properties of conductivity and stability in MOFs‐derived nanomaterials, they find applications as electrode materials in batteries or capacitors, [57] including the use of MOFs‐derived nanomaterials in electrocatalysis and electrochemical sensors [58,59] . Additionally, MOFs‐derived nanomaterials are also widely used in the field of photocatalysis.…”