Precision spectroscopy of atomic systems 1 is an invaluable tool for the advancement of our understanding of fundamental interactions and symmetries 2. Recently, highly charged ions (HCI) have been proposed for sensitive tests of physics beyond the Standard Model 2-5 and as candidates for high-accuracy atomic clocks 3,5. However, the implementation of these ideas has been hindered by the parts-per-million level spectroscopic accuracies achieved to date 6-8. Here, we cool a trapped HCI to the lowest reported temperatures, and introduce coherent laser spectroscopy on HCI with an eight orders of magnitude leap in precision. We probe the forbidden optical transition in 40 Ar 13+ at 441 nm using quantum-logic spectroscopy 9,10 and measure both its excited-state lifetime and g-factor. Our work ultimately unlocks the potential of HCI, a large, ubiquitous atomic class, for quantum information processing, novel frequency standards, and highly sensitive tests of fundamental physics, such as searching for dark matter candidates 11 or violations of fundamental symmetries 2. Alike a microscope aimed at the quantum world, laser spectroscopy pursues ever higher resolving power. Every increase in resolution enables deeper insights into the subtle effects that all known fundamental interactions have on the atomic wave function. Advances in optical frequency metrology have dramatically improved resolution in the last three decades 1 , and are making laser spectroscopy an extremely sensitive tool for studying open physics questions such as the nature of dark matter, the strength of parity violation, or a possible violation of Einstein's theory of relativity 2. However, only a few atomic and ionic species are currently within the reach of cutting-edge optical frequency metrology. Expanding this field of exploration to systems with high sensitivity to such effects is therefore crucial. Due to their extreme properties, highly charged ions (HCI) are promising candidates for such fundamental tests. Contributions from special