Perfect absorption and strong coupling are two highly
sought-after
regimes of light–matter interactions. Both regimes have been
studied as separate phenomena in excitonic 2D materials, particularly
in MoS2. However, the structures used to reach these regimes
often require intricate nanofabrication. Here, we demonstrate the
occurrence of perfect absorption and strong coupling in thin MoS2 multilayers supported by a glass substrate. We measure reflection
spectra of mechanically exfoliated MoS2 flakes at various
angles beyond the light-line via Fourier plane imaging and spectroscopy
and find that absorption in MoS2 monolayers increases up
to 74% at the C-exciton by illuminating at the critical angle. Perfect
absorption is achieved for ultrathin MoS2 flakes (4–8
layers) with a notable angle and frequency sensitivity to the exact
number of layers. By calculating zeros and poles of the scattering
matrix in the complex frequency plane, we identify perfect absorption
(zeros) and strong coupling (poles) conditions for thin (<10 layers)
and thick (>10 layers) limits. Our findings reveal rich physics
of
light–matter interactions in bare MoS2 flakes, which
could be useful for nanophotonic and light harvesting applications.