Grid shells supporting transparent or opaque panels are largely used to cover long-spanned spaces because of their lightness, the easy setup, and economy. This paper presents the results of experimental static and dynamic investigations carried out on a large-scale freeform grid shell mock-up, whose geometry descended from an innovative Voronoi polygonal pattern. Accompanying finite-element method (FEM) simulations followed. To these purposes, a four-step procedure was adopted: (1) a perfect FEM model was analyzed; (2) using the modal shapes scaled by measuring the mock-up, a deformed unloaded geometry was built, which took into account the defects caused by the assembly phase; (3) experimental static tests were executed by affixing weights to the mockup, and a simplified representative FEM model was calibrated, choosing the nodes stiffness and the material properties as parameters; and (4) modal identification was performed through operational modal analysis and impulsive tests, and then, a simplified FEM dynamical model was calibrated. Due to the high deformability of the mockup, only a symmetric load case configuration was adopted