New dual‐beam leaky‐wave radiations based on spoof surface plasmon polariton (SSPP) waveguide, in which the amplitude, radiation, angle and polarization of each beam can be designed independently, is proposed. The proposed SSPP waveguide is made of a corrugated metallic strip with bilateral 45°‐tilted grooves, whose surface impedance is flexibly designed by changing the depth of grooves. To realize dual‐beam leaky‐wave radiations, the surface impedance of SSPP waveguide is modulated periodically based on the superposition theory of aperture fields. By simply adjusting the modulation factors, modulation periods, and initial phase differences of the modulated surface impedance, the amplitude, radiation angle, and polarization of each beam can be further controlled independently as well. The results have been validated by both numerical simulations and experimental measurements, which show good agreement with the theoretical predictions.