Asymmetric Synthesis of Six‐Membered Ring Nitrogen Heterocycles with More Than One Heteroatom

Mátyus, Péter; Tapolcsányi, Pál

doi:10.1002/9783527625505.ch7

Asymmetric Synthesis of Nitrogen Heterocycles 2009

DOI: 10.1002/9783527625505.ch7

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Asymmetric Synthesis of Six‐Membered Ring Nitrogen Heterocycles with More Than One Heteroatom

Péter Mátyus¹,

Pál Tapolcsányi²

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Cited by 3 publications

References 246 publications

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A Unified Strategy Toward 5‐, 6‐, and 7‐Membered Nitrogen Heterocycles Through Free Radical then Metal‐Mediated Functionalization of Ene‐carbamates

et al. 2017

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Free-radical carbo-alkenylation of N-aryl, N-benzyl, and N-phenethyl-ene-carbamates with a disulfone provides vinylsulfones which may then be functionalized and engaged in Heck-type coupling to furnish highly substituted 5-, 6-and 7-membered nitrogen heterocycles. Grignardmediated cyclization starting from the same substrates further allowed a nucleophilic cascade process, affording a straightforward access to hydrocarbazoles, which may be regarded as potent intermediates for the synthesis of alkaloids of the aspidosperma family.

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A Unified Strategy Toward 5‐, 6‐, and 7‐Membered Nitrogen Heterocycles Through Free Radical then Metal‐Mediated Functionalization of Ene‐carbamates

et al. 2017

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ChemInform Abstract: Asymmetric Synthesis of Six‐Membered Ring Nitrogen Heterocycles with More than One Heteroatom

Mátyus¹,

Tapolcsányi²

2010

ChemInform

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Asymmetric nucleophilic dearomatization of diazarenes by anion-binding catalysis

2016

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The first anion-binding organocatalyzed enantioselective Reissert-type dearomatization of diazarenes has been developed. This reaction represents a synthetic challenge since diazarenes have various reactive sites. The use of a chiral tetrakistriazole as a C-H-based hydrogen-donor catalyst allowed the straightforward highly regio- and enantioselective synthesis of a variety of chiral diazaheterocycles.

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Asymmetric Synthesis of Six‐Membered Ring Nitrogen Heterocycles with More Than One Heteroatom

Cited by 3 publications

References 246 publications

A Unified Strategy Toward 5‐, 6‐, and 7‐Membered Nitrogen Heterocycles Through Free Radical then Metal‐Mediated Functionalization of Ene‐carbamates

A Unified Strategy Toward 5‐, 6‐, and 7‐Membered Nitrogen Heterocycles Through Free Radical then Metal‐Mediated Functionalization of Ene‐carbamates

ChemInform Abstract: Asymmetric Synthesis of Six‐Membered Ring Nitrogen Heterocycles with More than One Heteroatom

Asymmetric nucleophilic dearomatization of diazarenes by anion-binding catalysis

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