2024
DOI: 10.1021/acsestair.4c00070
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Atmospheric Oxidation of PFAS by Hydroxyl Radical: A Density Functional Theory Study

Michael R. Dooley,
Steven P. Nixon,
Benjamin E. Payton
et al.

Abstract: Per- and polyfluoroalkyl substances (PFAS) are persistent, widely spread, and harmful pollutants. They can travel through the air, be transformed by radicals, and deposit into water or onto surfaces. They enter the atmosphere via direct emission, degradation of precursors, or aerosol formation. A recent investigation found novel compounds in rainwater, meaning PFAS may undergo transformations in the atmosphere. These transformations might exhibit distinct behavior compared to more well-researched reactions, cr… Show more

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