2017
DOI: 10.1103/physrevb.95.224301
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Attenuation process of the longitudinal phonon mode in a TeO2 crystal in the 20-GHz range

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“…The relatively large error bars for the TA2 at high temperatures are due to the weak signal intensity resulting from the partial absorption of 532 nm light at around 300 K; at lower temperatures, the signal intensity increases because the absorption edge shifts to the shorter wavelength on cooling. While the hardening of phonons on cooling is an ordinary behavior, 39,40) the softening of the LA mode on cooling is somewhat unusual, which is not covered in the previous measurements conducted at higher temperatures. 27) The temperature dependences of n and/or r can be the origin of this apparent softening (frequency decrease), but it is not compatible with the hardening of the TA modes, the identical n and/or r values are relevant.…”
Section: Resultsmentioning
confidence: 85%
“…The relatively large error bars for the TA2 at high temperatures are due to the weak signal intensity resulting from the partial absorption of 532 nm light at around 300 K; at lower temperatures, the signal intensity increases because the absorption edge shifts to the shorter wavelength on cooling. While the hardening of phonons on cooling is an ordinary behavior, 39,40) the softening of the LA mode on cooling is somewhat unusual, which is not covered in the previous measurements conducted at higher temperatures. 27) The temperature dependences of n and/or r can be the origin of this apparent softening (frequency decrease), but it is not compatible with the hardening of the TA modes, the identical n and/or r values are relevant.…”
Section: Resultsmentioning
confidence: 85%