Balanced IR Nonlinear Optical Performance Achieved by Cation–Anion Module Cosubstitution in V-Based Salt-Inclusion Oxychalcogenides
Mao-Yin Ran,
Sheng-Hua Zhou,
Bing-Xuan Li
et al.
Abstract:Oxychalcogenides have become notable contenders for infrared nonlinear optical (IR NLO) applications because of their diverse heteroanionic functional motifs. However, while the main group elements are well-explored for these motifs, transition elements have been less studied and lack high-performance materials. To address this gap, we investigated a series of noncentrosymmetric [Ba 4 (Ba 6 S)][(VO x S 4−x ) 6 ] (space group: P6 3 ), the first V-based salt-inclusion oxychalcogenides demonstrating phase-matched… Show more
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