Bi-chromatic driver enabled control of high harmonic generation in atomic targets

Abstract

We investigated the high-order harmonic generation by interacting time-delayed, linearly polarized bi-chromatic laser pulses with the atomic target. The frequency ratio of secondary to primary fields ($\omega_2/\omega_1$), along with the carrier-envelope-phase (CEP) and respective time-delay between the two pulses, are very instrumental in controlling the ionization of the electron and so the quantum dynamics in continuum. We observed an optimum CEP ($\phi$) and time delay ($t_d$) for a given bi-chromatic frequency ratio, giving maximum cutoff energy. We studied the effect of CEP and time delay for fixed frequency ratio and observed that the harmonic cutoff could be controlled in an experimentally feasible way. Moreover, the harmonic yield in the energy range 140 eV $-$ 240 eV is also calculated, and it is observed that the harmonic yield scales as $\propto -\phi^{5/6}$. The attosecond pulses for different CEP is also calculated by superposing the harmonics in the same energy range, and $\sim 200$ as pulses are observed with peak intensity decreasing with CEP, following the variation of respective harmonic yield with CEP.

Control over the secondary collision of electron in high-order harmonic generation

“…Numerous investigations have been conducted to explore the influence of the CEP of the laser pulse on various properties of the generated harmonic spectra. These studies have examined effects such as enhancing the intensity of the spectral continuum [44,54], extending and regulating the harmonic cutoff [3,55], CEP-dependent frequency modulations in harmonic spectra [56], and the role of CEP in electron quantum paths [57][58][59]. Similarly, there is substantial research focused on electron multiple recollision dynamics, wherein a small percentage of the ionized electron wavepacket may revisit the parent ion more than once before recombining with it [60][61][62][63][64][65].…”