Bioinspired and biomimetic nucleobase-containing polymers: the effect of selective multiple hydrogen bonds

Yao, Nan; Wu, Jiang; Liu, Guangming; Hua, Zan

doi:10.1039/d4sc06720g

Chem. Sci.

2024

DOI: 10.1039/d4sc06720g

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Bioinspired and biomimetic nucleobase-containing polymers: the effect of selective multiple hydrogen bonds

Nan Yao,

Jiang Wu,

Guangming Liu

et al.

Abstract: Inspired by the selective multiple hydrogen bonds of complementary nucleobases in nucleic acids, robust nucleobase-containing polymers/materials have been developed through high-efficient and scalable step-growth or chain polymerizations.

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Complementary Nucleobase‐Containing Double‐Network Elastomers with High Energy Dissipation and Room‐Temperature Fast Recovery

Zeng,

Wu,

Hua

et al. 2024

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Elastomers have been widely employed in various industrial products such as tires, actuators, dampers, and sealants. While various methods have been developed to strengthen elastomers, achieving continuously high energy dissipation with fast room‐temperature recovery remains challenging, prompting the need for further structural optimization. Herein, high energy dissipated and fast recoverable double‐network (DN) elastomers are fabricated, in which the supramolecular polymers of complementary adenine and thymine serve as the first network and the covalently cross‐linked soft polymer as the second network. Both networks are efficiently prepared via photopolymerization. The resulting DN elastomer displays high energy dissipation and room temperature fast recovery, which can be attributed to the good independence of supramolecular and covalent networks. Furthermore, it is demonstrated that the DN elastomer can be exploited as excellent cushioning materials under continuous impacts. This work presents a feasible avenue for fabricating DN elastomers with high energy dissipation and fast recovery based on the multiple hydrogen bonds of complementary nucleobases.

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Complementary Nucleobase‐Containing Double‐Network Elastomers with High Energy Dissipation and Room‐Temperature Fast Recovery

Zeng,

Wu,

Hua

et al. 2024

Small

View full text Add to dashboard Cite

show abstract

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Bioinspired and biomimetic nucleobase-containing polymers: the effect of selective multiple hydrogen bonds

Abstract: Inspired by the selective multiple hydrogen bonds of complementary nucleobases in nucleic acids, robust nucleobase-containing polymers/materials have been developed through high-efficient and scalable step-growth or chain polymerizations.

Cited by 1 publication

References 118 publications

Complementary Nucleobase‐Containing Double‐Network Elastomers with High Energy Dissipation and Room‐Temperature Fast Recovery

Complementary Nucleobase‐Containing Double‐Network Elastomers with High Energy Dissipation and Room‐Temperature Fast Recovery

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