2022
DOI: 10.1002/ange.202200420
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Bioinspired Total Synthesis of Erectones A and B, and the Revised Structure of Hyperelodione D

Abstract: The field of biomimetic synthesis seeks to apply biosynthetic hypotheses to the efficient construction of complex natural products. This approach can also guide the revision of incorrectly assigned structures. Herein, we describe the evolution of a concise total synthesis and structural reassignment of hyperelodione D, a tetracyclic meroterpenoid derived from a Hypericum plant, alongside some biogenetically related natural products, erectones A and B. The key step in the synthesis of hyperelodione D forms six … Show more

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