The purpose of this study was to develop a rapid and green method for the synthesis of lignocelluloses-based materials with superior mechanical properties. Samples were produced by hot-pressed method using different concentrations of CaCO3 and poly (methyl methacrylate) particles-filled nanolignocelluloses composites which was synthesized through mechano-chemical method. Poly (methyl methacrylate) and CaCO3 nanoparticles have been used as nanofillers. Bending strength, elasticity modulus, and dimensional stability, thermal properties of the developed lignocelluloses-based composites were determined. In view of the experimental results, it is found that the composites materials have good mechanical, dimensional stability, and thermal properties which enhanced as the filler loading increased. Thus, herein described lignocelluloses-based materials showed important characteristics to be concluded that these composites are suitable to be used for the design of flooring and construction systems.