We investigate the generation, characterization and measurement of non-classical correlations and entanglement in ultracold atomic gases. Specifically, we propose new tests to demonstrate non-classical correlations, Einstein-Podolsky-Rosen (EPR) entanglement and Bell inequality violations, in systems involving dilute gas Bose-Einstein condensates (BECs). We focus on the challenges of generating and preserving these correlations in atom-optics schemes with massive particles and define appropriate operational measurements to demonstrate them experimentally. Further, we characterize how measures of EPR entanglement and violations of a Bell inequality evolve with time and scale with system size.To begin, we detail a theoretical proposal to demonstrate the well-known optical HongOu-Mandel (HOM) effect of destructive quantum interference with massive particles. Our proposed matter-wave experiment, realized recently in a related experimental setup [Lopes et. al., Nature 520, 66 (2015)], utilizes pair-correlated atoms produced via spontaneous fourwave mixing in colliding BECs. The atom pairs are then subjected to Bragg pulses -the atom-optics equivalent of optical mirrors and beam-splitters -to realize a HOM atom interferometer. By taking advantage of the multimode nature of the four-wave mixing process we formulate a measurement protocol which, unlike the optical case, does not require repeated measurements for different beam-splitter settings. We perform numerical simulations of a realistic experimental system and predict a HOM 'dip' visibility of ∼ 69%, indicating the correlations between atom pairs are stronger than classically allowed.In Chapter 5 we outline a theoretical proposal to demonstrate a violation of a motionalstate Bell inequality with massive particles. Identically to Chapter 4, the proposal uses pairs of momentum-entangled atoms produced via spontaneous four-wave mixing in colliding BECs. However, this scheme requires two pairs of atoms which are used as the input state of an atom-optics analog of the Rarity-Tapster interferometer, constructed via a sequence of Bragg pulses. We formulate a measurable form of the Clauser-Horne-Shimony-Holt (CHSH) Bell inequality taking into account experimental limitations, and perform numerical simulations of a realistic experimental system for a range of parameters. We predict values of the CHSH-Bell parameter up to S 2.5, demonstrating a violation of the CHSH-Bell inequality which is bounded by S ≤ 2 for local hidden-variable theories.In Chapter 6 we investigate the prospect of demonstrating EPR entanglement between massive particles via spin-changing collisions in a spinor BEC. This investigation is motivated by recent experimental work of Gross et al. [Nature 480, 219 (2011)] who reported inconclusive results in an attempt to measure EPR entanglement. In the experiment, spinchanging collisions between atoms in the (F, m F ) = (2, 0) state lead to pairs of strongly correlated atoms being created in opposing (F, m F ) = (2, ±1) states. For m F = ±1 states in...