2024
DOI: 10.1021/acscatal.4c01557
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Boosting the Urea Synthesis Rate on Ni Single-Atom Catalysts: The Impact of Acetonitrile Electrolyte in the Tandem CO2 Reduction/Nucleophilic Addition Reaction

Peize Li,
Yan Wei,
Xiaoju Yang
et al.

Abstract: The tandem CO 2 reduction reaction (CO 2 RR) process/nucleophilic addition reaction can be an efficient and environmentally friendly method for the synthesis of urea. However, the low stability of the CO 2•− intermediates causes a low yield of urea through the nucleophilic addition reaction. Here, we propose an effective method to improve the yield of nucleophilic addition to synthesize urea on Ni single-atom catalysts (Ni-SACs) by introducing acetonitrile into aqueous electrolytes. A high yield of urea of 1.1… Show more

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