Bound-state electrons synergy over photochromic high-crystalline C3N5 nanosheets in enhancing charge separation for photocatalytic H2 production

Shen, Yu; Du, Xin; Shi, Yuxing; Nguetsa Kuate, Loic Jiresse; Chen, Zhouze; Zhu, Cheng; Tan, Lei; Guo, Feng; Li, Shijie; Shi, Weilong

doi:10.1016/j.apmate.2024.100202

Advanced Powder Materials

2024

DOI: 10.1016/j.apmate.2024.100202

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Bound-state electrons synergy over photochromic high-crystalline C3N5 nanosheets in enhancing charge separation for photocatalytic H2 production

Yu Shen,

Xin Du,

Yuxing Shi

et al.

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Cited by 9 publications

References 61 publications

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Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H₂ Evolution

Jing,

Wang,

Hao

et al. 2024

Advanced Sustainable Systems

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With the advantages of large specific surface area and high porosity of general metal‐organic frame materials, russian blue analogs have broad application prospects in catalysis. In this work, a series of ultra‐thin N‐doped carbon coated Fe‐CoP (Fe‐CoP@NC) are prepared by phosphating Fe‐Co‐Co Prussian blue analogs (Fe‐Co‐Co PBA) in different degrees for the broad‐spectrum photocatalytic hydrogen evolution. The results show that Fe‐CoP@NC‐3 has the highest photocatalytic hydrogen production rate of 16.6 mmol h−1 g−1, which is 83 times greater than that of Fe‐Co‐Co PBA. The excellent stability of Fe‐CoP@NC‐3 is proved by cyclic experiments. The outstanding photocatalytic H2 production activity of Fe‐CoP@NC‐3 can be ascribed to the strong electron coupling effect between Fe‐CoP and N‐doped carbon layer. The photogenerated electrons of Fe‐CoP are transferred to the N‐doped carbon layer, which is electron transport mediator accelerating the electron transfer and synergetic improving the hydrogen evolution efficiency. This work provides an effective strategy for designing an ultra‐thin N‐doped carbon layer coated phosphide photocatalyst with strong electron coupling effect.

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Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H₂ Evolution

Jing,

Wang,

Hao

et al. 2024

Advanced Sustainable Systems

View full text Add to dashboard Cite

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Heteroatom doping in 2D MXenes for energy storage/conversion applications

Sahoo,

Kumar,

Hussain

et al. 2024

Advanced Powder Materials

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Incorporation of hydroxyl groups and π-rich electron domains into g-C3N4 framework for boosted sacrificial agent-free photocatalytic H2O2 production

Shen,

Shi,

Wang

et al. 2024

Chemical Engineering Journal

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Bound-state electrons synergy over photochromic high-crystalline C3N5 nanosheets in enhancing charge separation for photocatalytic H2 production

Cited by 9 publications

References 61 publications

Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H₂ Evolution

Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H₂ Evolution

Heteroatom doping in 2D MXenes for energy storage/conversion applications

Incorporation of hydroxyl groups and π-rich electron domains into g-C3N4 framework for boosted sacrificial agent-free photocatalytic H2O2 production

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About

Bound-state electrons synergy over photochromic high-crystalline C3N5 nanosheets in enhancing charge separation for photocatalytic H2 production

Cited by 9 publications

References 61 publications

Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H2 Evolution

Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H2 Evolution

Heteroatom doping in 2D MXenes for energy storage/conversion applications

Incorporation of hydroxyl groups and π-rich electron domains into g-C3N4 framework for boosted sacrificial agent-free photocatalytic H2O2 production

Contact Info

Product

Resources

About

Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H₂ Evolution

Strong Electron Coupling Effect of Prussian Blue Analogs Derived Ultrathin Nitrogen‐Doped Carbon Wrapped Fe‐CoP for Enhanced Wide Spectrum Photocatalytic H₂ Evolution