Brazilian Atmospheric Inventories – BRAIN: a comprehensive database of air quality in Brazil

Abstract

Abstract. Developing air quality management systems to control the impacts of air pollution requires reliable data. However, current initiatives do not provide datasets with large spatial and temporal resolutions for developing air pollution policies in Brazil. Here, we introduce the Brazilian Atmospheric Inventories (BRAIN), the first comprehensive database of air quality and its drivers in Brazil. BRAIN encompasses hourly datasets of meteorology, emissions, and air quality. The emissions dataset includes vehicular emissions derived from the Brazilian Vehicular Emissions Inventory Software (BRAVES), industrial emissions produced with local data from the Brazilian environmental agencies, biomass burning emissions from FINN – Fire INventory from the National Center for Atmospheric Research (NCAR), and biogenic emissions from the Model of Emissions of Gases and Aerosols from Nature (MEGAN) (https://doi.org/10.57760/sciencedb.09858, Hoinaski et al., 2023a; https://doi.org/10.57760/sciencedb.09886, Hoinaski et al., 2023b). The meteorology dataset has been derived from the Weather Research and Forecasting Model (WRF) (https://doi.org/10.57760/sciencedb.09857, Hoinaski and Will, 2023a; https://doi.org/10.57760/sciencedb.09885, Hoinaski and Will, 2023c). The air quality dataset contains the surface concentration of 216 air pollutants produced from coupling meteorological and emissions datasets with the Community Multiscale Air Quality Modeling System (CMAQ) (https://doi.org/10.57760/sciencedb.09859, Hoinaski and Will, 2023b; https://doi.org/10.57760/sciencedb.09884, Hoinaski and Will, 2023d). We provide gridded data in two domains, one covering the Brazilian territory with 20×20 km spatial resolution and another covering southern Brazil with 4×4 km spatial resolution. This paper describes how the datasets were produced, their limitations, and their spatiotemporal features. To evaluate the quality of the database, we compare the air quality dataset with 244 air quality monitoring stations, providing the model's performance for each pollutant measured by the monitoring stations. We present a sample of the spatial variability of emissions, meteorology, and air quality in Brazil from 2019, revealing the hotspots of emissions and air pollution issues. By making BRAIN publicly available, we aim to provide the required data for developing air quality policies on municipal and state scales, especially for under-developed and data-scarce municipalities. We also envision that BRAIN has the potential to create new insights into and opportunities for air pollution research in Brazil.​​​​​​​