GaN-based high-electron-mobility transistors (HEMTs) have emerged as a promising candidate for next-generation high-efficiency power electronics including high-frequency power amplifiers and high-voltage power switches. [1] However, reliability problems such as gate leakage current and current collapse are the main issues that limit the performance of AlGaN/GaN HEMTs. [2] The common way to reduce the current collapse of devices is to grow a SiN x as a passivation layer. [3] Nevertheless, a detrimental rise in leakage current may be caused by fabrication damages. [4,5] Remote inductively coupled plasma chemical vapor deposition (ICP-CVD) [6] and low-pressure chemical vapor deposition (LPCVD) [7] techniques have been proposed for damage-free passivation. However, these techniques require longer time, higher cost, and higher temperature. [1] It is still a challenge to obtain lower gate leakage and lower current collapse simultaneously.